This video is for “This Head I Hold (Version 2)” from Electric Guest.  I was initially interested because this track, and in fact Electric Guest’s whole debut album, Mondo, is produced by Danger Mouse.  Now, I am a fan of both the track and the video.  

As Complex points out,

It should be noted that lead singer Asa Taccone is the younger brother of Jorma Taccone from The Lonely Island, and was the composer of their Grammy winning SNL number “Dick In A Box” with Justin Timberlake. 

Explains the sense of humor in the video.

(Source: complex.com)